COMPARISON OF PRODUCT QUALITY ESTIMATION OF PROPYLENE POLYMERIZATION IN LOOP REACTORS USING ARTIFICIAL NEURAL NETWORK MODELS
DOI:
https://doi.org/10.11113/jt.v78.9279Keywords:
Artificial neural network, soft sensor, propylene polymerizationAbstract
One of the major challenges in polymerization industry is the lack of online instruments to measure polymer end-used properties such as xylene soluble, particle size distribution and melt flow index (MFI). As an alternative to the online instruments and conventional laboratory tests, these properties can be estimated using model based-soft sensor. This paper presents models for soft sensors to measure MFI in industrial polypropylene loop reactors using artificial neural network (ANN) model, serial hybrid neural network (HNN) model and stacked neural network (SNN) model. All models were developed and simulated in MATLAB. The simulation results of the MFI based on the ANN, HNN, and SNN models were compared and analyzed. Â The MFI was divided into three grades, which are A (10-12g/10 min), B (12-14g/10 min) and C (14-16 g/10 min). The HNN model is the best model in predicting all range of MFI with the lowest root mean square error (RMSE) value, 0.010848, followed by ANN model (RMSE=0.019366) and SNN model (RMSE=0.059132). The SNN model is the best model when tested with each grade of the MFI. It has shown lowest RMSE value for each type of MFI (0.012072 for MFI A, 0.017527 for MFI B and 0.015287 for MFI C), compared to HNN model (0.014916 for MFI A, 0.041402 for MFI B and 0.046437 for MFI C) and ANN model (0.015156 for MFI A, 0.076682 for MFI B, and 0.037862 for MFI C).
References
Kim, M., Lee, Y.H., Han, I.S., and Han, C. 2005. Clustering Based Hybrid Soft Sensor for an Industrial Polypropylene Process with Grade Changeover Operation. Ind. Eng. Chem. Res. 44: 334-342.
Peacock, A. J. 2000. Handbook of Polyethylene: Structures, Properties, and Applications. New York: Marcel Dekker.
Latado, A., Embirucu, M., Neto, A. G., & Pinto, J. C. 2001. Polymer Modelling: Modelling of End Use Properties of Poly (propylene/ethylene) Resins. Polymer Testing. 20: 419-439.
Zhang, J.,Qi, B.X., and Yong, M. 2006. Inferential Estimation of Polymer Melt Index Using Sequentially Trained Aggregated Neural Network. Chem. Eng. Technol. 44: 442-448.
Ghasem, N.M., Sata, S.A., and Hussain, M.A. . 2007. Temperature Control of a Bench-Scale Batch Polymerization Reactor for Polystyrene Production. Chem. Eng. Technol. 30(9): 1193–1202.
Fernandes, F. A. N. and Lona, L. M. F. 2005. Neural Network Applications in Polymerization Processes. Braz. J. Chem. Eng. 22(3): 401-418.
Azaman, F., Azid, A., Juahir, H., Mohamed, M., Yunus, K., Toriman, M. E., & Hairoma, N. 2015. Application of Artificial Neural Network and Response Surface Methodology for Modelling of Hydrogen Production Using Nickel Loaded Zeolite. Jurnal Teknologi. 77(1): 109-118.
Dashtbayazi, M. R., & Ghanbarian, M. 2015. Comparison of Artificial Neural Network Methods in Modeling of Polymer Matrix Composite Turning. Mechanical Engineering. 47(2).
Hinchliffe, M., Montague, G., and Willis, M. 2003. Hybrid Approach to Modeling an Industrial Polyethylene Process. AIChE Journal. 49(12): 3127-3137.
Jian S., Xinggao L., and Youxian S. 2006. Melt Index Prediction by Neural Network Based in Independent Component Analysis and Multi-Scale Analysis. Neurocomputing. 70(2006): 280-287.
Xia, L., and Pan, H. 2010. Inferential Estimation of Polypropylene Melt Index Using Stacked Neural Network Based on Absolute Error Criteria. International Conference on Computer, Mechatronics, Control and Electronic Engineering. (2010): 216-218.
Gonzaga, J.C.B., Meleiro, L.A.C., Kiang, C., and Maciel Filho, R. 2009. ANN-based Soft-Sensor for Real-Time Process Monitoring and Control of An Industrial Polymerization Process. Computer and Chemical Engineering. 33(2009): 43-49.
Albizzati, E., Giannini, U., Collina, G., Noristi, L., and Resconi, L. 1996. Catalyst and Polymerizations. In Moore, E. P. (Ed.) Polypropylene Handbook. New York: Hanser Publisher. (): 11-111.
Zacca, J. J. and Ray, W. H. 1993. Modelling of The Liquid Phase Polymerization of Olefins in Loop Reactors. Chemical Engineering Science. 48(22): 3743-3765.
Lucca, E. A., Filho, R. M., Melo, P. A., and Pinto, J. C. 2008. Modeling and Simulation of Liquid Phase Propylene Polymerizations in Industrial Loop Reactors. Macromolecular Symposia. 271: 8-14.
Harun, N. F. 2009. Formulation of Modeling and Simulation Algorithm for Propylene Homopolymerization in Industrial Loop Reactors. M. Eng. Project Report, Skudai. Malaysia: Universiti Teknologi Malaysia.
Jamaludin, M. Z. 2009. Modelling The Product Quality and Production Rate Of Propylene Polymerization In Industrial Loop Reactors. M.Eng. dissertation, Malaysia: Universiti Teknologi Malaysia.
Wolpert, D.H. 1992. Stacked Generalization. Neural Networks. 5: 241-259.
Sridhar, D. V., Seagrave, R. C., and Bartlett, E. B. 1996. Process Modeling Using Stacked Neural Networks. AIChE Journal. 42(9): 2529-2539.
Downloads
Published
Issue
Section
License
Copyright of articles that appear in Jurnal Teknologi belongs exclusively to Penerbit Universiti Teknologi Malaysia (Penerbit UTM Press). This copyright covers the rights to reproduce the article, including reprints, electronic reproductions, or any other reproductions of similar nature.