SPATIAL AND TEMPORAL BEHAVIOR OF PB, CD, AND ZN RELEASE DURING SHORT TERM LOW INTENSITY RESUSPENSION EVENTS
DOI:
https://doi.org/10.11113/jt.v80.9748Keywords:
Heavy metal contaminated sediment, resuspension, Pb, Cd and Zn release, spatial and temporal releaseAbstract
Sediment as the largest storage and resources of heavy metal plays an important role in the metal remobilisation and release. Continuous particulate matter in suspension increased the level and mobility of metals, of which poses a serious problem particularly to aquatic organisms. The purpose of this research is to investigate the fate and amount of contaminant released through sediment resuspension by using particle entrainment simulator (PES) with low turbulence intensity. The heavy metal release from sediment mixture of sand/silt/clay with percentage of 90/5/5, respectively was studied. In particular, the research paid attention to the contaminant release at the early resuspension stage (i.e. within 3 hr resuspension) by reviewing the metal releases of Zn, Cd and Pb in water column at five elevations from the bed of PES. Results showed that the concentration of remobilised heavy metal during resuspension event for Cd, Zn and Pb was in ranged of 0.034 to 0.139 mg/L, 0.014 to 0.071 mg/L and 0.007 to 0.029 mg/L respectively. The affinities of heavy metal release discussed in this study was Cd > Zn > Pb. Concentrations of the heavy metal fluctuated within the water column and have the lowest values at near bed. The highest concentration observed for Cd and Zn was at one integral length scale from the sediment bed and at t = 120 mins. Even at low turbulence intensity, the heavy metal release was still observed and is significant to the water quality.
References
Ankley, G., Di Toro, D., Hansen, D., Berry, W. 1996. Technical Basis and Proposal for Deriving Sediment Quality Criteria for Metals. Environmental Toxicology and Chemistry. 15: 2056-2066.
Atkinson, C. a, Jolley, D. F. & Simpson, S. L. 2007. Effect of Overlying Water pH, Dissolved Oxygen, Salinity and Sediment Disturbances on Metal Release and Sequestration from Metal Contaminated Marine Sediments. Chemosphere. 69(9): 428-37.
Banu, Z., Chowdhury, M. S. A., Hossain, M. D. & Nakagami, K. 2013. Contamination and Ecological Risk Assessment of Heavy Metal in the Sediment of Turag River, Bangladesh: An Index Analysis Approach. Journal of Water Resource and Protection. 239-248.
Borglin, S., Wilke, A., Jepsen, R. & Lick, W. 1996. Parameters Affecting the Desorption of Hydrophobic Organic Chemicals from Suspended Sediments. Env. Toxic. Chem. 15: 2254-2262.
Cantwell, M. G., Burgess, R. M. 2004. Variability of Parameters Measured During the Resuspension of Sediments with a Particle Entrainment Simulator. Chemosphere. 56: 51-58.
Cappuyns, V., Swennen, R. & Verhulst, J. 2004. Assessment of Acid Neutralizing Capacity and Potential Mobilisation of Trace Metals from Land-disposed Dredged Sediments. The Science of the Total Environment. 333(1-3): 233-47.
Eggleton, J. & Thomas, K. V. 2004. A Review of Factors Affecting the Release and Bioavailability of Contaminants during Sediment Disturbance Events. Environment international. 30(7): 973-80.
Hopfinger, E. J., Toly, J. A. 1976. Spatially Decaying Turbulence and Its Relation to Mixing Across Density Interfaces. J. Fluid Mech. 78: 155-175.
Huang, J., Ge, X., Yang, X., Zheng, B. & Wang, D. 2012. Remobilization of Heavy Metals during the Resuspension of Liangshui River Sediments Using an Annular Flume. Chinese Science Bulletin. 57(27): 3567-3572.
Ghrefat, H., and Yusuf, N. 2006. Assessing Mn, Fe, Cu, Zn, and Cd Pollution in Bottom Sediments of Wadi Al-Arab Dam, Jordan. Chemosphere. 65: 2114-2121
Nguyen, H. L., Leermakers, Mca, Osán, J., Török, S. & Baeyens, W. 2005. Heavy Metals in Lake Balaton: Water Column, Suspended Matter, Sediment and Biota. The Science of the Total Environment. 340(1-3): 213-30.
Miller, M. C., Mc Cave, I. N., and Komar, P. D. 1977. Threshold of Sediment Motion under Unidirectional Current. Sedimentology. 24: 507-527.
Reible, D., Fleeger, J., Pardue, J., Tomson, M., Kan, A. & Thibodeaux, L. 2002. Contaminant Release during Removal and Resuspension. http://www. hsrc.org/hsrc/html/ssw/ssw-contaminant.html.
Simpson, S. L., Angel, B. M. & Jolley, D. F. 2004. Metal Equilibration in Laboratory-contaminated (Spiked) Sediments Used for the Development of Whole-Sediment Toxicity Tests. Chemosphere. 54(5): 597-609.
Salomons, W, Stigliani, W. M. 1995. Biogeodynamics of Pollutants in Soils and Sediments. Springer-Verlag Berlin Heidelberg. 198-199.
Tsai, C. H., & Lick, W. 1985. A Portable Device for Measuring Sediment Suspension. Dept. of Mechanical and Environmental Engineering, University of California, Santa Barbara, CA.
Van Den Berg, C., Merks, A. & Duursma, E. 1987. Organic Complexation and Its Control of the Dissolved Concentrations of Copper and Zinc in the Scheldt Estuary. Est., Coas. and Shelf Sci. 24: 785-797.
Van Rijn, L. C. 2007. Unified View of Sediment Transport by Currents and Waves. II: Suspended Transport. J. Hydr. Eng. 133(6): 668-689.
Yap, C. K., Ismail, A. & Tan, S.G. 2004. Heavy Metal (Cd, Cu, Pb and Zn) Concentrations In the Green-lipped mussel Perna viridis (Linnaeus) Collected from Some Wild and Aquacultural Sites in the West Coast of Peninsular Malaysia. Food Chemistry. 84: 569-575.
Yi, Y., Yang, Z. & Zhang, S. 2011. Ecological Risk Assessment of Heavy Metals in Sediment and Human Health Risk Assessment of Heavy Metals in Fishes in the Middle and Lower Reaches of the Yangtze River Basin. Environmental Pollution. 159(10): 2575-2585.
Yu, K. C., Tsai, L. J., Chen, S. H., and Ho, S.T. 2001. Chemical Binding of Heavy Metals in Anoxic River Sediments. Water Research. 35(17): 4086-4094.
Wei, Y. L. and Huang, Y. L. 1998. Behaviour of Sequential Extraction of Lead from Thermally Treated Lead (II) Doped Alumina. J. Environ. Qual. 27: 343-348.
Downloads
Published
Issue
Section
License
Copyright of articles that appear in Jurnal Teknologi belongs exclusively to Penerbit Universiti Teknologi Malaysia (Penerbit UTM Press). This copyright covers the rights to reproduce the article, including reprints, electronic reproductions, or any other reproductions of similar nature.